Phonon renormalization of the N\`{e}el transition in KCuF$_{3}$
ORAL
Abstract
Critical magnetic fluctuations in the one-dimensional antiferromagnet KCuF$_3$, in the form of diffuse scattering around the magnetic (001) Bragg peak, have been studied with resonant soft x-ray scattering. Using x-rays near the Cu L$_{3}$ edge to exploit the 2\textit{p} $\to$ 3\textit{d} dipole transition, the (001) was directly observed at temperatures ranging from 23K to above the transition temperature (T$_{N}$ $\approx$ 43K). Notably, the phase transition exhibits hysteresis, with T$_{N}$ sensitive to whether the sample was cooled or heated prior to measurement. This suggests that the phase transition is weakly first order, as might be expected by a transition renormalized by phonons. The temperature dependence of the coherence length and the diffuse scattering, as well as the role played by Jahn-Teller phonons in the transition are discussed.
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Authors
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James Lee
University of Illinois, Urbana-Champaign, Frederick Seitz Materials Research Laboratory, University of Illinois
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S. Yuan
University of Illinois, Urbana-Champaign
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A. Rusydi
National University of Singapore
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Serban Smadici
University of Illinois, Urbana-Champaign, Frederick Seitz Materials Research Laboratory, University of Illinois
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S.L. Cooper
University of Illinois, Urbana-Champaign
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Eduardo Fradkin
University of Illinois, Urbana-Champaign, University of Illinois, UIUC
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P. Abbamonte
University of Illinois, Urbana-Champaign, Dept of Physics, Seitz Materials Research Lab, Frederick Seitz Materials Research Laboratory, University of Illinois