Magnetic Diffuse Scattering in the Frustrated Kagome Antiferromagnet YBaCo$_{4}$O$_{7}$

ORAL

Abstract

Cobalt oxides of composition RBaCo$_{4}$O$_{7}$ (R=Y, Tb-Lu) crystallize with a lattice structure topologically related to that of the pyrochlore. Considering only the magnetic transition metal sublattice, R-114 appears as Kagome sheets linked by triangular layers and is therefore expected to provide a new materials class for exploring geometric magnetic frustration. We have recently shown that stoichiometric R-114 compound orders antiferromagnetically into a long-range ordered (LRO) structure with features common to the $\sqrt 3 \ast \sqrt 3$ negative chirality spin arrangements often found in Kagome net systems. In contrast, small excesses of O added to the system, as little as 0.1, destroys this LRO state. To explore the nature of the frustrated magnetism in this novel system, we have measured magnetic diffuse scattering on YBaCo$_{4}$O$_{7}$ and YBaCo$_{4}$O$_{7.1}$ single crystals at the ISIS facility. Large maps of reciprocal space in several planes have been recorded showing a very structured diffuse scattering. The data compared to models obtained by the Monte-Carlo method using the metropolis algorithm, reveal the exact nature of the disordered ground state in this new class of frustrated magnets.

Authors

  • Pascal Manuel

    ISIS Facility, Rutherford Appleton Laboratory

  • Laurent Chapon

    ISIS Facility, Rutherford Appleton Laboratory, ISIS, Rutherford Appleton Laboratory, ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, UK, ISIS Facility, STFC-RAL, Didcot,OX110QX, UK

  • Paolo Radaelli

    ISIS Facility, Rutherford Appleton Laboratory

  • John Mitchell

    Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave, Argonne IL 60439, Mat. Sci. Div., ANL, Argonne National Laboratory, Materials Science Division, Argonne National Laboratory, LANL, Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USA, Argonne Natl Lab, Materials Science Division, Argonne National Laboratory, Argonne, IL, Argonne National Lab

  • H. Zheng

    Argonne National Laboratory, Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave, Argonne IL 60439