Magnetic domains in multiferroic YMn$_$2O$_5$ probed by Spherical Neutron Polarimetry under electric field

ORAL

Abstract

Precise determination of the magnetic structures in multiferroics RMn$_2$O$_5$ (R: Y, Ho, Bi) have been obtained by single crystal neutron diffraction. The analysis shows the presence of zig-zag antiferromagnetic chains in the ab-plane. An additional weak magnetic component parallel to the c-axis was detected which is modulated in phase quadrature with the a-b components. The nature and population of the coexisting antiferromagnetic domains in YMn$_2$O$_5$ have been determined by Spherical Neutron Polarimetry under an external electric field. We have proved that reversing the electrical polarity results in the inversion of the population of two types of antiferromagnetic domains, with opposite in-plane spin components. This analysis strongly supports theories in which the coupling of the magnetic configuration to the ferroelectric polarisation is due to magnetic exchange striction and likely not related to the small cycloidal modulation in the bc-plane.

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Authors

  • Carlo Vecchini

    ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, UK

  • Laurent Chapon

    ISIS Facility, Rutherford Appleton Laboratory, ISIS, Rutherford Appleton Laboratory, ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, UK, ISIS Facility, STFC-RAL, Didcot,OX110QX, UK

  • Paolo Radaelli

    ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, UK

  • Aziz Daoud-Aladine

    ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, UK

  • Jane Brown

    Institut Laue-Langevin, 6, rue Jules Horowitz, BP156-38042 Grenoble Cedex 9 - France

  • Tapan Chatterji

    Institut Laue-Langevin, 6, rue Jules Horowitz, BP156-38042 Grenoble Cedex 9 - France

  • S. Park

    Rutgers Univ., Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA

  • S.-W. Cheong

    Rutgers University, RCEM and Rutgers University, Piscataway, NJ, Rutgers University (Deparment of Physics), Rutgers Univ., Department of Physics and Astronomy, Rutgers University, Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA, Rutgers Center for Emergent Materials and Department of Physics \& Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA, Rutgers Center for Emergent Materials and Department of Physics \& Astronomy, Rutgers University, Piscataway, New Jersey 08854