Neutron Scattering Study of Magnetic and Orbital Order in MnV$_{2}$O$_{4}$

ORAL

Abstract

Neutron diffraction and inelastic scattering has been used to study the spinel system MnV$_{2}$O$_{4}$. The results confirm the existence of two phase transitions. The first, near 56 K, is from a paramagnetic state to a collinear ferrimagnetic phase. There is a second simultaneous structural and magnetic transition at 53 K to a tetragonal structure with a non-collinear ferrimagnetic state. The low T magnetic structure has been definitively resolved, and is seen to be associated with a gap in the magnetic excitation spectrum. The magnetic structure is compatible with a staggered orbital ordering.Inelastic scattering has been carried out using both triple axis and time of flight techniques, and several branches of magnetic excitations are visible. These observations put tight constraints on theoretical models for MnV$_{2}$O$_{4}$. An initial account of some of the results of this work appears in arXiv:0711.1844v1.

Authors

  • Stephen Nagler

    Oak Ridge National Laboratory, Oak Ridge TN 37831, Oak Ridge National Laboratory

  • Ovidiu Garlea

    Neutron Scattering Science Division, ORNL, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge national laboratory, Oak Ridge National Laboratory

  • Ronying Jin

    Materials Science and Technology Division, ORNL, Oak Ridge, TN 37831 and Univ. of Tennessee, Knoxville, TN 37996, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge TN 37831, Oak Ridge National Laboratory

  • David Mandrus

    Materials Science and Technology Division, ORNL, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge, TN 37831, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge TN 37831, Oak Ridge Natl Lab

  • Doug Abernathy

    Oak Ridge National Laboratory

  • Bertrand Roessli

    Paul Scherrer Institute

  • Martha Miller

    Argonne National Laboratory

  • Arthur Schultz

    Argonne National Lab (IPNS), Argonne National Laboratory

  • Qingzhen Huang

    NIST Center for Neutron Research, NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, National Institute of Standards and Technology (NCNR)

  • C.D. Frost

    Rutherford-Appleton Laboratories, ISIS Facility, RAL