Nanoscale ferromagnetism and doping effect in manganites

ORAL

Abstract

We investigated temperature variation of ferromagnetic (FM) microstructures in La$_{1-x}$Sr$_{x}$MnO$_{3}$ (x=0.175) by low-temperature Lorentz microscopy. Also, changes of the FM domain structures by substituting non-magnetic Al$^{3+}$ ion for Mn one were examined. We succeeded in observing changes of magnetic domain structures from large FM domains with the average width of 1$\mu $m to stripe-shaped FM ones with the 100nm width in the metallic phase. On the other hand, the insulator phase was found in La$_{1-x}$Sr$_{x}$Mn$_{1-y}$Al$_{y}$O$_{3}$ (x=0.175, y=0.02). We found that the insulating phase exhibits a characteristic bi-modal distribution of the FM domains, which is characterized as the coexisting state of distinct types of the FM domains; one is the stripe-shaped FM domains and the other is the plate-shaped one. This mixture of distinct types of the FM domains breaks the coherence of the conductivity and results in the insulating character in La$_{1-x}$Sr$_{x}$Mn$_{1-y}$Al$_{y}$O$_{3}$ (x=0.175, y=0.02). In addition, we found the nanoscale FM domains around the rhombohedral-to-orthorhombic structural transition temperature in La$_{1-x}$Sr$_{x}$Mn$_{1-y}$Al$_{y}$O$_{3}$ (x=0.175, y=0.04).

Authors

  • S. Mori

    Osaka Prefecture University

  • K. Yoshidome

    Osaka Prefecture University

  • Y. Horibe

    Rutgers Univ., Rutgers University

  • T. Asaka

    NIMS

  • Y. Matsui

    Superconducting Materials Center, National Institute for Materials Science, 1-2-1, Sengen, Tsukuba, Ibaraki, NIMS

  • K. Takenaka

    Nagoya Univrsity