Bond-stretching phonon mode in stripe ordered orthorhombic $\bf Nd_{1.67}Sr_{0.33}NiO_4$.

ORAL

Abstract

Inelastic x-ray scattering (IXS) experiments on $\rm Nd_{1.67} Sr_{0.33}NiO_4$ have been performed to study electron-phonon interactions in this charge stripe ordered nickelate. Resurgent interest in such phenomena has been triggered by recent results on the high temperature superconductors, where a kink in the electron dispersion as well as striking anomalies in high- energy optical phonon modes have been observed. A significant softening of the bond-stretching-phonon mode for $\rm Q||[100]$ was also observed in the tetragonal nickelate $\rm La_{1.69}Sr_ {0.31}NiO_4$ with inelastic neutron scattering. Moreover, this compound shows an apparent splitting of the bond-stretching mode along the $\rm [110]$ direction. Here we present first IXS results for $\rm Q||[110]$ on the orthorhombic compound $\rm Nd_ {1.67}Sr_{0.33}NiO_4$, which is characterized by domains with unidirectional stripe order. By probing different spots on the sample with different domain distribution, a weak contrast between the phonon spectra has been observed. We discuss these differences in terms of phonons propagating parallel and perpendicular to the stripe direction, as well as the anisotropic, i.e. orthorhombic, lattice structure.

Authors

  • M. H\"ucker

    Brookhaven National Laboratory

  • T. Fukuda

    Japan Atomic Energy Research Institute (JAERI), SPring-8

  • Genda Gu

    Brookhaven National Laboratory, 1. Brookhaven National Laboratory, USA, Physics Department, Brookhaven National Laboratory, Upton, New York 11973, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973

  • John Tranquada

    Brookhaven National Laboratory, Brookhaven National Lab

  • A. Q. R. Baron

    Japan Synchrotron Radiation Research Institute (JASRI), SPring-8

  • J.P. Hill

    Brookhaven National Laboratory