Electronic reconstruction at SrMnO$_{3}$-LaMnO$_{3}$ superlattice interfaces

ORAL

Abstract

Progress in molecular beam epitaxy made possible the growth of manganese oxide superlattices with the dopant ions arranged in separate regular layers. Little is known about how this ``structural'' doping is reflected into the MnO$_{2}$ planes; for instance what is the plane effective hole concentration. We studied superlattices made of SrMnO$_{3}$ and LaMnO$_{3}$ layers with a doping of x=0.33 using resonant soft x-ray scattering. For scattering momenta at which the non-resonant contribution is suppressed by symmetry, i. e. L=3 in units of the superlattice period, resonant soft x-ray scattering probes the distribution of doped holes, and, in particular, the nature of the interface between the doped and undoped layers. Our measurements at the O K edge show a temperature-dependent hole distribution. This electronic reconstruction which occurs with cooling below T$_{c}$ =220~K is related to the transition of the superlattice to a ferromagnetic state. Resonant scattering spectra at the Mn L edges from spin and orbital distributions have complex shapes providing additional insights into these new materials.

Authors

  • Serban Smadici

    Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, IL 61801, USA

  • Peter Abbamonte

    Dept. of Physics, F. Seitz Materials Research Laboratory, University of Illinois, Urbana-Champaign, Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, IL 61801, USA, University of Illinois

  • Anand Bhattacharya

    Materials Science Division, Argonne National Laboratory, Materials Science Division (MSD), Argonne National Laboratory (Argonne), Argonne National Laboratory, IL 60439, USA

  • Xiaofang Zhai

    FS MRL, UIUC, IL 61801, USA, F. Seitz Materials Research Laboratory, University of Illinois, Urbana, IL

  • James Eckstein

    University of Illinois, Urbana, Department of Physics and F Seitz Materials Research Laboratory, University of Illinois, Urbana, Department of Physics and Fredrick Seitz Materials Research Laboratory, University of Illinois, Urbana, FS MRL, UIUC, IL 61801, USA, University of Illinois at Urbana Champaign, Department of Physics and Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, IL 61801, Department of Physics, University of Illinois at Urbana-Champaign

  • Andrivo Rusydi

    University of Hamburg, University of Hamburg, D-20355, Germany