Thickness dependence of the structural, magnetic, and electronic, properties of epitaxial La$_{0.5}$Sr$_{0.5}$CoO$_{3}$ films on SrTiO$_{3}$(001) substrates

Bulk La$_{1-x}$Sr$_{x}$CoO$_{3}$ (LSCO) materials have received considerable attention due to the existence of spin-state transitions, magnetoelectronic phase separation, and giant anomalous Hall effect. In our prior work we have established optimized conditions for the deposition of high quality epitaxial LSCO thin films. In this work, we provide a comprehensive study of the variation of structural, morphological, magnetic, and electronic properties as a function of film thickness. This investigation has been carried out as a controlled function of oxygen stoichiometry using the total sputtering pressure (30, 70, and 140 mTorr, at an O$_{2}$ / Ar ratio of 0.4) as the control parameter. High resolution WAXRD, x-ray rocking curves, x-ray reflectivity, AFM, d.c. magnetometry, and electronic transport measurements have all been employed. Our results indicate that the thickness dependence of the electronic and magnetic properties is dominated by the sensitive interplay between oxygen stoichiometry and strain relaxation. The behavior at very low thickness is discussed in terms of the known phenomenology of the magnetoelectronic phase separation in this material.