Tuning Physical Properties via Isovalent Doping in Ba$_{2-x}$Sr$_{x}$CoO$_{4}$

ORAL

Abstract

It is known that monoclinic Ba$_{2}$CoO$_{4}$ is an antiferromagnetic (AFM) insulator with Neel temperature $T_{N}$=25K. We found that isovalent Sr substitution for Ba drastically changes the structural and magnetic properties of Ba$_{2-x}$Sr$_{x}$CoO$_{4}$ system. With increasing $x$, $T_{N}$ initially increases then decreases after reaching the maximum at $x$=0.5. Correspondingly, its crystal structure changes from monoclinic ($x<$0.5) to orthorhombic ($x\ge $0.5) at room temperature. The correlation between structure and physical properties will be discussed.

Authors

  • Hao Sha

    Department of Physics, Florida International University, Miami, FL 33199

  • Jiandi Zhang

    Florida International University, Department of Physics, Florida International University, Miami, FL 33199

  • Q. Huang

    NIST Center for Neutron Research, NIST Center for Neutron Research, Gaithersburg, Maryland 20899

  • V.O. Garlea

    Oak Ridge National Laboratory, ORNL, Oak Ridge National Laboratory, Oak Ridge, TN 37831

  • Brian Sales

    Oak Ridge National Laboratory, Oak Ridge TN 37831, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge, TN 37831

  • David Mandrus

    Oak Ridge National Laboratory, Oak Ridge TN 37831, Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee, Oak Ridge National Laboratory, Oak Ridge National Lab., Materials Science and Technology Division, Oak Ridge, TN, Oak Ridge National Laboratory, Oak Ridge, TN 37831

  • Rongyin Jin

    ORNL, Oak Ridge National Laboratory, Oak Ridge National Laboratory, Oak Ridge, TN 37831