Thermal expansion measurements in multiferroic HoMn$_{2}$O$_{5}$

ORAL

Abstract

Thermal expansion measurements were done on HoMn$_{2}$O$_{5}$ along the a,b,and c axes at zero applied magnetic field. Distinctive anomalies in the linear expansivities along the principal axes were seen at T$_{N}$=44K,T$_{C}$=39K,T$_{N\mbox{'}}$=20K and T$_{C\mbox{'}}$=15K with a notable negative c-axis thermal expansivity below 100K.All three axes were observed to shrink at T$_{N}$ and T$_{N\mbox{'}}$ while a and b expand as c shrinks when it passes through T$_{C}$ and T$_{C\mbox{'}}$ upon cooling. These anomalies are intimately correlated with anomalies in the dielectric constant and the specific heat at the phase transition temperatures. Our observations suggest that the coupling of the magnetic orders with the dielectric properties are mediated by strong magnetoelastic effects and the lattice anomalies play a crucial role in understanding the ferroelectricity in the compound. The anomalies associated with the ferroelectric transitions at T$_{C}$ and T$_{C\mbox{'}}$ show a thermal hysteresis revealing the first order nature of the transitions.

Authors

  • Clarina dela Cruz

  • Fei Yen

  • Bernd Lorenz

  • C.W. Chu

    Texas Center for Superconductivity and Advanced Materials, University of Houston, Houston, TX 77204-5002, Hong Kong University of Science and Technology; Texas Center for Superconductivity, University of Houston; Lawrence Berkeley National Laboratory, Dept. of Physics and TcSUH, University of Houston, Houston,TX 77204-5002, Department of Physics and TCSAM, University of Houston

  • M.M. Gospodinov

    Institute of Solid State Physics, Bulgarian Academy of Sciences, 1784 Sofia, Bulgaria