Low-temperature Resonant Ultrasound Spectroscopy on Alpha-Pu

POSTER

Abstract

We measured the elastic constants of polycrystalline Alpha-plutonium (16 atoms per unit cell) as a function of temperature (18-350K) using Resonant Ultrasound Spectroscopy$^{1}$. A smooth behavior in the temperature dependence of the elastic moduli curves is found, with no evidence for any electronic, magnetic or structural phase transitions. The data can be fit by the quasiharmonic Einstein-oscillator model. The high-temperature bulk modulus yields an anharmonic Gr\"{u}neisen parameter gamma of 5.1, and the low-temperature elastic constants results a Debye temperature $\Theta _{D}$ of about 205K$^{2}$. [1] Albert Migliori and John Sarrao, ``Resonant Ultrasound Spectroscopy,'' John Wiley {\&} Sons, INC 1997 [2] A. Migliori, H. Ledbetter, J. Betts, M. Ramos, S. Harrington, and S. El-Khatib, to be submitted to Physical Review B, 2004

Authors

  • Sami El-Khatib

    New Mexico State University

  • P. DeChatel

    New Mexico State University, European Commission, Joint Research Center, Institute for Transuranium Compounds, LANSCE, Los Alamos National Laboratory, Physics Department, Colorado State University, School of Electrical and Computer Engineering, Purdue University

  • Albert Migliori

    Los Alamos National Laboratory

  • H. Ledbetter

    Los Alamos National Laboratory

  • J. Betts

    Los Alamos National Laboratory

  • S. Harrington

    Los Alamos National Laboratory