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Measure of temperature and ionization in warm dense mid-Z metal alloys using x-ray absorption spectroscopy

POSTER

Abstract

Warm dense matter exists at temperatures of order 10 eV and a few times solid density, where the complex balance of collective and quantum effects precludes standard approximations used in plasma physics or condensed matter physics. Understanding ionization in the warm dense matter regime, in particular\, is an active area of research that requires additional experimental data to benchmark and improve current predictive capabilities. In this study, we present the experimental results and analysis of K-shell x-ray absorption spectra. X-ray absorption is used to extract an inference of the charge state distribution and electron temperature. Targets comprised of copper, brass, and copper-aluminum were uniformly heated to temperatures 10–40 eV and compressed to densities of 5–25 g/cm3. The variation in the fraction of copper allows for exploration of density variations on ionization. The experiments were conducted at the OMEGA laser facility using a buried layer of copper, or copper alloy, tamped by plastic on both sides. The two sides were then irradiated by symmetric laser pulses and probed by a laser-generated x-ray source. Experimental results are compared to collisional-radiative models, where we find large discrepancies in the predicted x-ray absorption spectra at these conditions. We also explore the role of including density effects in the underlying atomic data used in the collisional-radiative models and compare the results to our experimental data.

Presenters

  • Tanner Cordova

    University of California San Diego

Authors

  • Tanner Cordova

    University of California San Diego

  • Mike J MacDonald

    Lawrence Livermore National Laboratory

  • Edward V Marley

    Lawrence Livermore National Laboratory, Laboratory for Laser Energetics

  • David Alexander Chin

    University of Rochester, Laboratory for Laser Energetics, Laboratory for Laser Energetics, University of Rochester, Rochester, NY, United States

  • Tilo Doeppner

    Lawrence Livermore National Laboratory

  • Richard A London

    Lawrence Livermore National Laboratory

  • Veronika K Kruse

    Lawrence Livermore National Laboratory

  • Howard A Scott

    Lawrence Livermore National Laboratory

  • Farhat N Beg

    University of California, San Diego

  • Federica Coppari

    Lawrence Livermore National Laboratory

  • Jim A Emig

    Lawrence Livermore Natl Lab

  • Stephanie B Hansen

    Sandia National Laboratories

  • Carolyn C Kuranz

    OCC

  • Marius Millot

    Lawrence Livermore National Laboratory

  • Philip M Nilson

    Laboratory for Laser Energetics (LLE)

  • Michael Springstead

  • Philip A Sterne

    Lawrence Livermore National Laboratory