Interband and intraband electron kinetics in non-thermal warm dense gold

ORAL

Abstract

Single-state warm dense matter may be produced via isochoric heating of thin metal foils using ultrafast high-power lasers. Previous experiments have confirmed that electron temperatures exceed ion temperatures during the initial picoseconds following excitation; however, electron kinetics in non-thermal states preceding establishment of a well-defined electron thermal distribution remain little understood. X-ray and optical probing techniques provide necessary resolution to investigate these electronic properties. Here, we will present a study of electron kinetics in warm dense gold produced by irradiating free-standing 30 nm Au foils with a 400 nm FWHM, 45 fs Ti:Sapphire laser system at SLAC National Accelerator Laboratory. The temporal evolutions of AC conductivity for 400 nm and 800 nm laser pulses are simultaneously determined with sub-100 fs resolution, providing insight into the 5$d$-6$s$/$p$ interband and 6$s/p$ intraband transitions respectively. Our results suggest that Auger decay and three-body recombination play important roles in electron thermalization of warm dense gold.

Authors

  • Shaughnessy Brennan Brown

    SLAC National Accelerator Laboratory

  • Zhijiang Chen

    SLAC National Accelerator Laboratory

  • Chandra Curry

    SLAC National Accelerator Laboratory

  • Philippe Hering

    SLAC National Accelerator Laboratory

  • Matthias C. Hoffmann

    SLAC National Accelerator Laboratory

  • Andrew Ng

    University of British Columbia

  • Matthew Reid

    University of Northern British Columbia

  • Ying Y. Tsui

    University of Alberta

  • S. H. Glenzer

    SLAC National Accelerator Laboratory, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, SLAC