Optical nonlinearity in Ar and N$_{2}$ near the ionization threshold

ORAL

Abstract

We directly measure the nonlinear optical response of argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. These responses are fundamental to high intensity femtosecond filamentation. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in contrast with a previous measurement [Loriot \textit{et al.}, Opt. Express \textbf{17}, 13429 (2009)] and calculations [Bree et al., Phys. Rev. Lett. \textbf{106}, 183902 (2011)]. In addition, we are able to cleanly separate the electronic and rotational components of the nonlinear response in nitrogen. In both Ar and N$_{2}$, we observe the peak instantaneous index response scale linearly with the laser intensity until the point of ionization, whereupon it turns abruptly negative and $\sim$ constant, consistent with plasma generation. In addition, we show that the results of Loriot \textit{et al.} are traceable to two-beam coupling via a plasma grating, and \textit{not} nonlinearity saturation or negative response.

Authors

  • J.K. Wahlstrand

    University of Maryland

  • Y.-H. Cheng

    University of Maryland

  • Y.-H. Chen

    University of Maryland, College Park, University of Maryland

  • Howard Milchberg

    IREAP, University of Maryland, University of Maryland, College Park, University of Maryland