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Precise β-Decay Measurements of Long-Lived Fission Product <sup>111</sup>Ag

ORAL

Abstract

Our understanding of the fragment mass distributions following fission impacts many applications, including reactor-neutrino studies, nuclear forensics, and stockpile stewardship science. The γ-ray emissions following the β- decay of fission products provide a reliable signature that is often used to identify relative yields and distributions from fission. However, the uncertainties in the existing nuclear data for γ-ray intensities and β-decay branching ratios for some of the isotopes used in these applications range from 5-35%, which propagates to significant error contributions in fission-chain yield calculations. To address this issue, we have developed an experimental approach to precisely measure γ-ray branching ratios following the decay of long-lived fission products. We have identified 111Ag as vital isotope where the data can be significantly improved, and we prepared radioactive samples from the CARIBU facility for measurement with our established detection system at Texas A&M University. We will present high-precision results of absolute γ-ray intensities from the recent measurement of 111Ag, which were measured to ≤ 1%.

Presenters

  • Isabel E Hernandez

    UC Berkeley

Authors

  • Isabel E Hernandez

    UC Berkeley

  • Kay Kolos

  • Daniel E Hoff

  • Nicholas David Scielzo

  • Victor Iacob

    Texas A&M University College Station

  • Dan G. Melconian

    Texas A&M University College Station

  • Shree K Neupane

  • Daniel P Burdette

    Argonne National Laboratory

  • Khushi Bhatt

    Argonne National Laboratory

  • Jason Allan Clark

    Argonne National Laboratory

  • Biying Liu

    University of Notre Dame, Notre Dame

  • Brenden Longfellow

  • Peter Mueller

    Argonne National Laboratory

  • Claus M Müller-Gatermann

    Argonne National Laboratory, ANL

  • Andrea L Richard

    Ohio University, Facility for Rare Isotope Beams; Department of Physics and Astronomy, Ohio University

  • D. Santiago-Gonzalez

    Argonne National Laboratory

  • Guy Savard

    Argonne National Laboratory

  • Anton P Tonchev

  • Adrian A. Valverde

    Argonne National Laboratory

  • Louis Varriano

    University of Washington