Precise $\beta^{-}$- and $\gamma$-ray emission probabilities in the decay of $^{67}$Cu
ORAL
Abstract
The $^{67}$Cu radionuclide has a potential for wide applications in cancer therapy and SPECT imaging. However, important decay properties that impact those applications are determined from a single measurement that was carried out about 60 years ago and reported without any uncertainties [1]. We have performed new measurements using chemically-purified $^{67}$Cu sources, produced via the $^{68}$Zn($\gamma$,p) reaction [2], in conjunction with the $\gamma$-ray spectroscopy technique. Both single and $\beta\gamma$-coincidence experiments were carried out using LEPS ($\gamma$ rays) and PIPS ($\beta^{-}$ and CE) detectors. Absolute $\beta^{-}$ and $\gamma$-ray emission probabilities were determined and those were found to differ significantly compared to the previously adopted values. The details of those measurements will be presented and their impact on the application of $^{67}$Cu as a therapeutic radionuclide in cancer therapy, as well as on various production-reaction cross sections, will be discussed. \\[4pt] [1] H.T. Easterday, Phys. Rev. 91, 653 (1953).\\[0pt] [2] N.A. Smith, D.L. Bowers and D.A. Ehst, Appl. Radiat. Isot. 70, 2377 (2012).
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Authors
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Jun Chen
Argonne National Laboratory
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F.G. Kondev
Argonne National Laboratory, ANL-Argonne, USA
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Irshad Ahmad
Argonne National Laboratory
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Michael Carpenter
Argonne National Laboratory
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David Ehst
Argonne National Laboratory
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John Greene
Argonne National Laboratory
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Vakhtang Makarashivili
Argonne National Laboratory
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Nick Smith
Argonne National Laboratory
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Shaofei Zhu
Argonne National Laboratory