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Can a photon saturate an atom without being absorbed?

ORAL

Abstract

As a resonant photon passes through a cloud of two-level atoms, it weakly saturates the atomic transition, modifying the index of refraction of the cloud, which can be measured as a nonlinear cross-phase shift (XPS) on a second, off-resonant beam. In cases where a photon is observed at a detector on the far side of the cloud, one might conclude that it had not been absorbed and that there should therefore be no XPS. In our experiment on absorptive optical nonlinearities in cold $^{\mathrm{85}}$Rb, we use post-selection to isolate the phase shift imparted by a transmitted photon. We find that despite not having been absorbed, transmitted photons impart a significant fraction (0.77$+$/-0.17) of the nonlinear XPS of the average incident photon, raising questions about the relationship between atomic excitation, absorption, and scattering at the fully quantized level.

Authors

  • Josiah Sinclair

    Univ of Toronto

  • Daniela Angulo

    Univ of Toronto

  • Kyle Thompson

    Univ of Toronto

  • Kent Bonsma-Fisher

    National Research Council of Canada

  • Aephraim Steinberg

    Univ of Toronto