Obtaining the complex correlation functions of photo-double ionization in helium
COFFEE_KLATCH · Invited
Abstract
The three particle breakup in photo-double ionization of helium, in dipole approximation, is fully characterized by two complex correlation functions. I will present a method to obtain these functions from experiment. The method is particularly well suited for experiments with $4\pi$ imaging of the two emitted photoelectrons, or of one electron and the recoiling photoion, as in COLTRIMS experiments. With unpolarized light or linearly polarized radiation one obtains the absolute magnitudes of the two correlation functions and the cosine of their relative complex phase. From these quantities one can deduce all observables in this process except for the direction of the circular dichroism or any spin-related observables. With a circular component in the incoming radiation one also obtains the sine of the relative phase and the degree of circular polarization. I will also discuss the effect of nondipolar corrections and the prospects of obtaining information on the three additional correlation functions originating from quadrupolar contributions in the interaction.
–
Authors
-
Bertold Kr\"assig
Chemistry Division, Argonne National Laboratory