Photon-Induced Near Field Electron Microscopy: Theoretical and Experimental

ORAL

Abstract

4D electron microscopy utilizes a pulsed electron packet to image structural dynamics of nanomaterial, induced by an optical pulse, in real time. In the presence of nanostructures, electrons can directly interact with photons, and either gain or lose light quanta. This near field photon-electron interaction enables visualization of nanoscale particles and interfaces with enhanced contrast, and is termed photon-induced near field electron microscopy (PINEM). Here, we give an account of the theoretical and experimental results of PINEM. In particular, the time-dependent Schr\"odinger equation for electron packets in the nanostructure-scattered electromagnetic (near) field is solved to obtain the evolution of the incident electron packet into discrete momentum wavelets. The characteristic length and time scales of the halo of electron- photon coupling are discussed in the framework of Rayleigh and Mie scatterings, providing the dependence of the PINEM effect on size, polarization, material, and spatiotemporal localization.

Authors

  • Sang Tae Park

    California Institute of Technology

  • Milo Lin

    California Institute of Technology

  • Ahmed Zewail

    California Institute of Technology