Partial helical order in Fe$_{\mathrm{3}}$PO$_{\mathrm{7}}$
ORAL
Abstract
For most magnetic systems, a particular ground state is chosen at low enough temperatures. For partially ordered states, there exists an extended manifold of possible ordering wavevectors available, from which the system cannot pick a unique solution, and instead shows short range order. Partial order has been observed, for example, in the Skrymion-lattice hosting materials MnSi and Fe$_{\mathrm{1-x}}$Co$_{\mathrm{x}}$Si, and in the latter it was shown to be the precursor to the Skyrmion lattice phase. Polycrystalline iron phosphate oxide (Fe$_{\mathrm{3}}$PO$_{\mathrm{7}})$ has been previously shown to host nanosized antiferromagnetic helical domains, implying a large number of topological defects are present below T$_{\mathrm{N}} \quad =$ 163 K. Here we present Neutron Diffraction data on single crystal Fe$_{\mathrm{3}}$PO$_{\mathrm{7}}$ which definitively shows partial order as evidenced by a continuous ring of scattering instead of well-defined Bragg peaks. This can be understood in terms of the competition between J$_{\mathrm{1}}$ (nearest neighbor) and J$_{\mathrm{2}}$ (next nearest neighbor) interactions in a Heisenberg model, which produces a quasi-degenerate manifold of ordering wavevectors. The partial order appears to be linked to the presence of topological defects, but at this point the origin of the latter is not well understood.
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Authors
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Colin Sarkis
Colorado State University
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Michael Tarne
Colorado State University
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Huibo Cao
Oak Ridge National Lab
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James Neilson
Colorado State University, Colorado State Univ
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Kate A. Ross
Colorado State University