Using Fluctuation Microscopy to Detect The Medium Range Order in Disordered Materials

POSTER

Abstract

In this poster we present some results from our X-ray and optical fluctuation microscopy studies of disordered materials. Fluctuation microscopy is sensitive to any medium range order present in amorphous and disordered materials, and obtains this sensitivity by examining the spatial fluctuations in coherent diffraction scattering. The method derives this sensitivity because the normalized variance depends on pair-pair correlation functions and hence can be used to detect the subtle structural correlations. We are exploring two variations of the fluctuation microscopy idea. One promising approach, for varying the resolution function within the same scan, is to use an elliptical (or rectangular) probe-forming aperture. The idea is that diffraction data along the narrow slit direction corresponds to low-resolution ($i.e.$ large sample volumes), whereas diffraction data along the wide slit direction corresponds to high-resolution data ($i.e.$ small sample volumes). The (admittedly simplistic) idea is that all sampling resolutions between these two extrema can be found by tracing the diffraction data along the azimuthal angle corresponding to the desired aperture width. This approach may eliminate the need for taking a series of scans at different probe.

Authors

  • D. Kumar

    Graduate Student at Arizona State University

  • M. Treacy

    Arizona State University

  • Seth Putterman

    Department of Chemistry and Biochemistry, Arizona State University, Tempe, AZ 85287, USA, Department of Physics, Arizona State University, Tempe, AZ 85287, USA, College of Optical Sciences, University of Arizona, Colorado State University, University of Virginia, Auburn University, Northern Kentucky University, Utah Valley State College, Brigham Young University, Arizona State University, University of Amsterdam, New Mexico State university, University of Minesota, Pulse Field Facility, NHMFL, LANL, NM, Institute of Physics ASCR , Czech Republic, University of Minesota-Twin City, New Mexico State University, Director, Advanced Photon Source, Argonne National Lab, Australian Synchotron Source, Advanced Photon Source, Argonne National Lab, University of Arizona, U.S. Naval Research Laboratory, Wellesley College, Observatoire de Paris, France, Freie Universitat Berlin, Florida State Univ., Univ. Sci. Tech. China, Iowa State University, Lawrence Livermore National Laboratory, Mahabad Azad University, Carnegie Mellon University, Tempe Preparatory Academy, University of California, Los Angeles

  • Seth Putterman

    Department of Chemistry and Biochemistry, Arizona State University, Tempe, AZ 85287, USA, Department of Physics, Arizona State University, Tempe, AZ 85287, USA, College of Optical Sciences, University of Arizona, Colorado State University, University of Virginia, Auburn University, Northern Kentucky University, Utah Valley State College, Brigham Young University, Arizona State University, University of Amsterdam, New Mexico State university, University of Minesota, Pulse Field Facility, NHMFL, LANL, NM, Institute of Physics ASCR , Czech Republic, University of Minesota-Twin City, New Mexico State University, Director, Advanced Photon Source, Argonne National Lab, Australian Synchotron Source, Advanced Photon Source, Argonne National Lab, University of Arizona, U.S. Naval Research Laboratory, Wellesley College, Observatoire de Paris, France, Freie Universitat Berlin, Florida State Univ., Univ. Sci. Tech. China, Iowa State University, Lawrence Livermore National Laboratory, Mahabad Azad University, Carnegie Mellon University, Tempe Preparatory Academy, University of California, Los Angeles

  • Seth Putterman

    Department of Chemistry and Biochemistry, Arizona State University, Tempe, AZ 85287, USA, Department of Physics, Arizona State University, Tempe, AZ 85287, USA, College of Optical Sciences, University of Arizona, Colorado State University, University of Virginia, Auburn University, Northern Kentucky University, Utah Valley State College, Brigham Young University, Arizona State University, University of Amsterdam, New Mexico State university, University of Minesota, Pulse Field Facility, NHMFL, LANL, NM, Institute of Physics ASCR , Czech Republic, University of Minesota-Twin City, New Mexico State University, Director, Advanced Photon Source, Argonne National Lab, Australian Synchotron Source, Advanced Photon Source, Argonne National Lab, University of Arizona, U.S. Naval Research Laboratory, Wellesley College, Observatoire de Paris, France, Freie Universitat Berlin, Florida State Univ., Univ. Sci. Tech. China, Iowa State University, Lawrence Livermore National Laboratory, Mahabad Azad University, Carnegie Mellon University, Tempe Preparatory Academy, University of California, Los Angeles

  • Seth Putterman

    Department of Chemistry and Biochemistry, Arizona State University, Tempe, AZ 85287, USA, Department of Physics, Arizona State University, Tempe, AZ 85287, USA, College of Optical Sciences, University of Arizona, Colorado State University, University of Virginia, Auburn University, Northern Kentucky University, Utah Valley State College, Brigham Young University, Arizona State University, University of Amsterdam, New Mexico State university, University of Minesota, Pulse Field Facility, NHMFL, LANL, NM, Institute of Physics ASCR , Czech Republic, University of Minesota-Twin City, New Mexico State University, Director, Advanced Photon Source, Argonne National Lab, Australian Synchotron Source, Advanced Photon Source, Argonne National Lab, University of Arizona, U.S. Naval Research Laboratory, Wellesley College, Observatoire de Paris, France, Freie Universitat Berlin, Florida State Univ., Univ. Sci. Tech. China, Iowa State University, Lawrence Livermore National Laboratory, Mahabad Azad University, Carnegie Mellon University, Tempe Preparatory Academy, University of California, Los Angeles

  • Seth Putterman

    Department of Chemistry and Biochemistry, Arizona State University, Tempe, AZ 85287, USA, Department of Physics, Arizona State University, Tempe, AZ 85287, USA, College of Optical Sciences, University of Arizona, Colorado State University, University of Virginia, Auburn University, Northern Kentucky University, Utah Valley State College, Brigham Young University, Arizona State University, University of Amsterdam, New Mexico State university, University of Minesota, Pulse Field Facility, NHMFL, LANL, NM, Institute of Physics ASCR , Czech Republic, University of Minesota-Twin City, New Mexico State University, Director, Advanced Photon Source, Argonne National Lab, Australian Synchotron Source, Advanced Photon Source, Argonne National Lab, University of Arizona, U.S. Naval Research Laboratory, Wellesley College, Observatoire de Paris, France, Freie Universitat Berlin, Florida State Univ., Univ. Sci. Tech. China, Iowa State University, Lawrence Livermore National Laboratory, Mahabad Azad University, Carnegie Mellon University, Tempe Preparatory Academy, University of California, Los Angeles